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Episodes
Season 1 30 episodes
- E01 Mr. Big
- E02 Diplomat's Daughter
- E03 School Days
- E04 Our Man in Toyland
- E05 Now You See Him... Now You Don't
- E06 Washington 4, Indians 3
- E07 KAOS in CONTROL
- E08 The Day Smart Turned Chicken
- E09 Satan Place
- E10 Our Man in Leotards
- E11 Too Many Chiefs
- E12 My Nephew the Spy
- E13 Aboard the Orient Express
- E14 Weekend Vampire
- E15 Survival of the Fattest
- E16 Double Agent
- E17 Kisses for KAOS
- E18 The Dead Spy Scrawls
- E19 Back to the Old Drawing Board
- E20 All in the Mind
- E21 Dear Diary
- E22 Smart, the Assassin
- E23 I'm Only Human
- E24 Stakeout on Blue Mist Mountain
- E25 The Amazing Harry Hoo
- E26 Hubert's Unfinished Symphony
- E27 Ship of Spies (1)
- E28 Ship of Spies (2)
- E29 Shipment to Beirut
- E30 The Last One in is a Rotten Spy
Season 2 30 episodes
- E01 Anatomy of a Lover
- E02 Strike While the Agent is Hot
- E03 A Spy for a Spy
- E04 The Only Way to Die
- E05 Maxwell Smart, Alias Jimmy Ballantine
- E06 Casablanca
- E07 The Decoy
- E08 Hoo Done It
- E09 Rub-a-Dub-Dub . . .Three Spies in a Sub
- E10 The Greatest Spy on Earth
- E11 Island of the Darned
- E12 Bronzefinger
- E13 Perils in a Pet Shop
- E14 The Whole Tooth and . . .
- E15 Kiss of Death
- E16 It Takes One to Know One
- E17 Someone Down Here Hates Me
- E18 Cutback at CONTROL
- E19 The Man from YENTA
- E20 The Mummy
- E21 The Girls from KAOS
- E22 Smart Fit the Battle of Jericho
- E23 Where-What-How-Who Am I?
- E24 The Expendable Agent
- E25 How to Succeed in the Spy Business Without Really Trying
- E26 Appointment in Sahara
- E27 Pussycats Galore
- E28 A Man Called Smart (1)
- E29 A Man Called Smart (2)
- E30 A Man Called Smart (3)
Season 3 26 episodes
- E01 The Spy Who Met Himself
- E02 Viva Smart
- E03 Witness for the Persecution
- E04 The Spirit is Willing
- E05 Maxwell Smart, Private Eye
- E06 Supersonic Boom
- E07 One of Our Olives is Missing
- E08 When Good Fellows Get Together
- E09 Dr. Yes
- E10 That Old Gang of Mine
- E11 The Mild Ones
- E12 Classification: Dead
- E13 The Mysterious Dr. T
- E14 The King Lives?
- E15 The Groovy Guru
- E16 The Little Black Book (1)
- E17 The Little Black Book (2)
- E18 Don't Look Back
- E19 99 Loses CONTROL
- E20 The Wax Max
- E21 Operation Ridiculous
- E22 Spy, Spy, Birdie
- E23 Run, Robot, Run
- E24 The Hot Line
- E25 Die, Spy
- E26 The Reluctant Redhead
Season 4 26 episodes
- E01 The Impossible Mission
- E02 Snoopy Smart vs. the Red Baron
- E03 Closely Watched Planes
- E04 The Secret of Sam Vittorio
- E05 Diamonds Are a Spy's Best Friend
- E06 The Worst Best Man
- E07 A Tale of Two Tails
- E08 The Return of the Ancient Mariner
- E09 With Love and Twitches
- E10 The Laser Blazer
- E11 The Farkas Fracas
- E12 Temporarily Out of CONTROL
- E13 Schwartz's Island
- E14 One Nation Invisible
- E15 Hurray for Hollywood
- E16 The Day They Raided the Knights
- E17 Tequila Mockingbird
- E18 I Shot 86 Today
- E19 Absorb the Greek
- E20 To Sire, with Love (1)
- E21 To Sire, with Love (2)
- E22 Shock It to Me
- E23 Leadside
- E24 Greer Window
- E25 The Not-So-Great Escape (1)
- E26 The Not-So-Great Escape (2)
Season 5 26 episodes
- E01 Pheasant Under Glass
- E02 Ironhand
- E03 Valerie of the Dolls
- E04 Widow Often Annie
- E05 The Treasure of C. Errol Madre
- E06 Smart Fell on Alabama
- E07 And Baby Makes Four (1)
- E08 And Baby Makes Four (2)
- E09 Physician: Impossible
- E10 The Apes of Rath
- E11 Age Before Duty
- E12 Is This Trip Necessary?
- E13 Ice Station Siegfried
- E14 Moonlighting Becomes You
- E15 House of Max (1)
- E16 House of Max (2)
- E17 Rebecca of Funny-Folk Farm
- E18 The Mess of Adrian Listenger
- E19 Witness for the Execution
- E20 How Green Was My Valet
- E21 And Only Two Ninety-Nine
- E22 Smartacus
- E23 What's It All About, Algie?
- E24 Hello, Columbus - Goodbye, America
- E25 Do I Hear a Vaults?
- E26 I Am Curiously Yellow
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